High responsivity colloidal quantum dots phototransistors for low-dose near-infrared photodetection and image communication.

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Tác giả: Tong Chen, Bo Hou, Hong Ji, Benxuan Li, Meng Li, Renjun Liu, Wenlong Ming, Diyar Mousa Othman, Ying Tang, Yudi Tu, Mingfei Xiao, Shijie Zhan, Zuhong Zhang, Hang Zhou

Ngôn ngữ: eng

Ký hiệu phân loại: 809.008 History and description with respect to kinds of persons

Thông tin xuất bản: England : Light, science & applications , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 746794

The surging demand and adoption of infrared photodetectors (IRPDs) in sectors of imaging, mobile, healthcare, automobiles, and optical communication are hindered by the prohibitive costs of traditional IRPD materials such as InGaAs and HgCdTe. Quantum dots (QDs), especially lead chalcogenide (PbS) QDs, represent the next-generation low-bandgap semiconductors for near-infrared (NIR) detection due to their high optical absorption coefficient, tunable bandgap, low fabrication costs, and device compatibility. Innovative techniques such as ligand exchange processes have been proposed to boost the performance of PbS QDs photodetectors, mostly using short ligands like 1,2-ethanedithiol (EDT) and tetrabutylammonium iodide (TBAI). Our study explores the use of long-chain dithiol ligands to enhance the responsivity of PbS QDs/InGaZnO phototransistors. Long-chain dithiol ligands are found to suppress horizontal electron transport/leakage and electron trapping, which is beneficial for responsivity. Utilizing a novel ligand-exchange technique with 1,10-decanedithiol (DDT), we develop high-performance hybrid phototransistors with detectivity exceeding 10
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