Phenylene Cage Synthesized by Metal-mediated Assembly of Phenylene Macrocycle and its Piezofluorochromic Behavior.

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Tác giả: Xuan-Wen Chen, Qing-Song Deng, Yuan-Zhi Tan, Guanjun Xiao, Jiang-Feng Xing, Xi-Han Yu, Bing-Hui Zheng, Bo Zou

Ngôn ngữ: eng

Ký hiệu phân loại: 809.008 History and description with respect to kinds of persons

Thông tin xuất bản: Germany : Angewandte Chemie (International ed. in English) , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 747783

A phenylene macrocycle containing two meta-phenylene units positioned opposite each other was used as a building block to construct phenylene cages via platinum-mediated C-C coupling. A phenylene cage (PC[10]3), consisting of three phenylene macrocycle units, was successfully synthesized and thoroughly characterized using nuclear magnetic resonance (NMR) spectroscopy and single-crystal X-ray diffraction. PC[10]3 exhibited significant backbone strain and displayed bright blue emission with a quantum yield of 96%. Additionally, PC[10]3 exhibited a broader and more pronounced piezofluorochromic response compared to its macrocyclic unit, undergoing a distinct photoluminescence shift from blue to yellow-green under pressure. This work opens new avenues for designing and synthesizing hydrocarbon nanocages.
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