Establishing Thermodynamic Graphs of Nitrogenous Radical Cations Abstracting Hydrogen Atoms and Their Applications in Photoredox Reactions.

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Tác giả: Yi-Lin Hou, Chong-Shan Hu, Guang-Bin Shen, Xin-Hua Wang, Jun Yang, Xia Zhao, Xiao-Qing Zhu

Ngôn ngữ: eng

Ký hiệu phân loại:

Thông tin xuất bản: Switzerland : Molecules (Basel, Switzerland) , 2025

Mô tả vật lý:

Bộ sưu tập: NCBI

ID: 78395

Nitrogenous compounds have been extensively utilized as hydrogen atom transfer (HAT) catalysts in photoredox reactions, with nitrogenous radical cations being the actual hydrogen atom abstractors. Building upon our previous work, 120 thermodynamic graphs of nitrogenous radical cations abstracting hydrogen atoms, which encompass seven vital thermodynamic parameters, are designed and established to elucidate their redox characteristics. Furthermore, the applications of thermodynamic graphs to select appropriate photocatalysts, assess the feasibility of the HAT process, and diagnose the possible activation mechanism were discussed, which would enable the utilities of nitrogenous compounds as HAT catalysts or nitrogenous radical cations as hydrogen atom abstractors in photoredox reactions.
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